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Take Command is a 32-bit or 64-bit GUI application.
TCC and TCC/LE are 32-bit or 64-bit console (character-mode) applications.
All are designed to run under Windows XP (SP2 and later), Windows 2003, Windows Vista, Windows 2008, and Windows 7.
The 32-bit and 64-bit versions of Take Command and TCC are identical in features. The 64-bit versions are slightly faster and don't have to deal with the directory and registry remapping that Windows does with 32-bit apps running in 64-bit Windows. The 64-bit versions will also use slightly more memory.